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\title{GENERATING COMPLETE SETS OF BEYOND-VOIGT LINE-SHAPE PARAMETERS FOR THE HITRAN DATABASE: \\ DATASET STRUCTURE, TEMPERATURE-DEPENDENCIES, LINE-SHAPE MODEL}

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\author{\underline{\FirstName N. \LastName STOLARCZYK},
  \underline{\FirstName P. \LastName WCIS\L{}O}}
\address{Institute of Physics, Faculty of Physics, Astronomy and Informatics, Nicolaus Copernicus University in Toru\'n, ul Grudzi\k{a}dzka 5, 87-100 Toru\'n, Poland)}

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\author{\FirstName L.~S. \LastName ROTHMAN,
  \underline{\FirstName R. \LastName HARGREAVES},
  \underline{\FirstName I.~E. \LastName GORDON}
  }
\address{Harvard-Smithsonian Center for Astrophysics, Atomic and Molecular Physics Division, Cambridge, MA, USA}

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\fancyhead[C]{{\footnotesize \textit{HRMS, 28th Colloquium, Dijon, France,
  Aug. 28 - Sept. 1, 2023}}}
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\begin{document}

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The accurate characterization of collision-perturbed spectral lines from many molecular systems requires a profound understanding of the beyond-Voigt effects that influence the spectrum~\footnote{
\href{http://dx.doi.org/10.1016/j.jqsrt.2016.01.024}{doi:10.1016/j.jqsrt.2016.01.024},
P. Wcis\l{}o, I.E. Gordon, H. Tran, Y. Tan, S.-M. Hu, A. Campargue, S. Kassi, D. Romanini, C. Hill, R.V. Kochanov and L.S. Rothman, \textit{JQSRT},
\textbf{177}, 75-91, (2016).}. These effects are described by eight essential spectral line-shape parameters: pressure broadening and shift ($\gamma_0$ and $\delta_0$), their speed dependencies ($\gamma_2$ and $\delta_2$), the real and imaginary parts of the complex Dicke parameter ($\tilde{\nu}_{opt}^r$ and $\tilde{\nu}_{opt}^i$) and the complex line-mixing coefficient (y$^r$ and y$^i$). Accurate knowledge of the temperature dependencies of these parameters is crucial for spectroscopic investigations of terrestrial~\footnote{
\href{https://doi.org/10.1016/j.crhy.2005.09.005}{doi:10.1016/j.crhy.2005.09.005},
C.E. Miller, L.R. Brown, R.A. Toth, D.C. Benner, V. M. Devi, \textit{C R Phys},
\textbf{6}, 876-887, (2005).} and extraterrestrial~\footnote{
\href{https://doi.org/10.1016/0019-1035(89)90062-6}{doi:10.1016/0019-1035(89)90062-6},
W.M.H. Smith, C.P. Conner, J. Simon, W.V. Schempp, W. Macy, \textit{Icarus},
\textbf{81}, 429-440, (1989).} atmospheres.
\par
In my presentation, I will focus on the methodology employed to establish an extensive dataset of beyond-Voigt spectral line-shape parameters~\footnote{
\href{https://doi.org/10.1016/j.jqsrt.2020.107477}{doi:10.1016/j.jqsrt.2020.107477},
P. Wcis\l{}o, F. Thibault, N. Stolarczyk, H. J\'o\'zwiak, M. S\l{}owi\'nski, M. Gancewski, K. Stankiewicz, M. Konefa\l{}, S. Kassi, A. Campargue, Y. Tan, J. Wang, K. Patkowski, R. Ciury\l{}o, D. Lisak, R. Kochanov, L.S. Rothman, I.E. Gordon, \textit{JQSRT},
\textbf{260}, 107477, (2021).}. I will discuss interpolation and extrapolation schemes of the \textit{ab initio} data to provide entries for the entire datasets in the HITRAN database~\footnote{
\href{https://doi.org/10.1016/j.jqsrt.2021.107949}{doi:10.1016/j.jqsrt.2021.107949},
I.E. Gordon \textit{et al}, \textit{JQSRT},
\textbf{277}, 107949, (2022).}. I will introduce the double-power-law (DPL) temperature-dependence model~\footnote{
\href{https://doi.org/10.1016/j.jqsrt.2019.106676}{doi:10.1016/j.jqsrt.2019.106676},
N. Stolarczyk, F. Thibault, H. Cybulski, H. J\'o\'zwiak, G. Kowzan, B. Vispoel, I.E. Gordon, L.S. Rothman, R.R. Gamache, P. Wcis\l{}o, \textit{JQSRT},
\textbf{240}, 106676, (2020).}, which offers a universal, straightforward, and accurate structure for each of the six line-shape parameters. I will discuss a new beyond-Voigt line-shape profile recommended for the HITRAN database.
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