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\title{OZONE SPECTROSCOPY IN THE TERAHERTZ RANGE FROM HIGH-RESOLUTION SYNCHROTRON SOLEIL EXPERIMENTS COMBINED WITH FAR-INFRARED MEASUREMENTS AND
      \textit{AB INITIO} INTENSITY CALCULATIONS }

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\author{\underline{\FirstName V. \LastName TYUTEREV}}
\address{Tomsk State University, Tomsk, Russia; GSMA UMR CNRS 7331, Reims University, France}

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\author{\FirstName A. \LastName BARBE}
\address{GSMA UMR CNRS 7331, Reims University, France}

\author{\underline{\FirstName L. \LastName MANCERON}}
\address{Synchrotron SOLEIL, Beamline AILES, Saint-Aubin, France}

\author{\FirstName B. \LastName GROUIEZ}
\address{GSMA UMR CNRS 7331, Reims University, France }

\author{\FirstName S. \LastName TASHKUN}
\address{Institute of Atmospheric Optics SB RAN, Tomsk, Russia }

\author{{\FirstName J. \LastName BURGALAT},
\underline{\FirstName M. \LastName ROTGER}}
\address{GSMA UMR CNRS 7331, Reims University, France}



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\fancyhead[C]{{\footnotesize \textit{HRMS, 28th Colloquium, Dijon, France,
  Aug. 28 - Sept. 1, 2023}}}
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More than half of the of the outgoing longwave radiation from the Earth to space is located in the FIR part 
of the electromagnetic spectrum at wavelengths greater than 15 micron. Ozone is one of the most important 
atmospheric species in terms of the impact on the climate changes and human health. It has a strong absorption
in the MW, THz and FIR, though only a relatively restricted part of lines has been experimentally measured 
in these ranges, which are the most efficient ones for the synchrotron setup at the SOLEIL CNRS equipment, 
in terms of the brightness if the synchrotron radiation, sensitivity of measurements and S/N ratio. 
The experimental setup for the ozone SOLEIL project has been previously described
\footnote{\text{L.Manceron, A.Barbe, V.Tyuterev et al., Far infrared spectroscopy of the ozone molecule and its isotopomers between 50 and 800 cm$^{-1}$, ASA-HITRAN Conference, Reims, (2022)}}.
 In this work,
the analyses of the experimental spectra recorded at four different P*L products for the main ozone isotopologue
and the theoretical modeling based on an improved effective Hamiltonian for the line positions and \textit{ab initio} 
intensity calculations
\footnote{\href{https://doi.org/10.1063/1.4973977}{doi:10.1063/1.4973977},
V.Tyuterev, R. Kochanov, S. Tashkun, Accurate \textit{ab initio} dipole moment surfaces of ozone: First principle intensity predictions for rotationally resolved spectra in a large range of overtone and combination bands \textit{JCP},
\textbf{146(6)}, art.no. 064304 (2017),}
\footnote{\href{https://doi.org/10.1016/j.jqsrt.2021.107801}{doi:10.1016/j.jqsrt.2021.107801},
V.Tyuterev, A.Barbe, S.Mikhailenko, E.Starikova, Y. Babikov, Towards the intensity consistency of the ozone bands in the infrared range: \textit{ab initio} corrections to the S&MPO database  \textit{JQSRT},
\textbf{272}, art.no. 107801 (2021).}
will be presented. The results will be given for the simultaneous fit of 
the rotational band GS-GS , the hot band $\nu$$_2$-$\nu$$_2$ and the FIR $\nu$$_2$ band conducting to the overall weighted 
standard deviation of 0.8 for 13500 line positions, including all previously available MW and FIR data
and the original SOLEIL measurements providing experimental accuracy of 0.00005-0.0001 cm$^{-1}$ for the best lines.
The accuracy issues and possible improvements in the SMPO, GEISA and HITRAN databases for large Ka quantum numbers will be discussed.
Supports from the CNRS SOLEIL research center for the experimental setup (project N 20211156) and from the RSF project 19-12-00171-P for the theoretical work and data analyses are acknowledged.


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